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1 article(s) from Barrière, Frédéric

Trifluoromethyl-substituted tetrathiafulvalenes

Olivier Jeannin,
Frédéric Barrière and
Marc Fourmigué

Beilstein J. Org. Chem. 2015, 11, 647–658, doi:10.3762/bjoc.11.73

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Graphical Abstract

Scheme 1: Mesomeric forms of 1,3-dithiole rings substituted with EWG.

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Scheme 2: Investigated TTF derivatives bearing EWG.

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Scheme 3: Synthetic procedures to the CF₃-substituted 4bc, 1c and 2ac molecules.

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Scheme 4: Synthetic procedure to 3bc.

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Figure 1: Correlation between the first oxidation potential E_1/2 and the sum of the Hammet σ_meta parameters. ...

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Figure 2: Calculated frontier orbitals of geometry-optimized [B3LYP/6-31G(d)] model compounds TTF, TTF-CF₃, T...

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Figure 3: View of the 2ac molecule. Thermal ellipsoids are shown at the 50% probability level.

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Figure 4: View of the 2bc molecule. Thermal ellipsoids are shown at the 50% probability level.

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Figure 5: View of the two crystallographically independent 4bc molecules. Thermal ellipsoids are shown at the...

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Figure 6: View of the 3bc molecule. Note the disordered CF₃ groups as well as the CO₂Me group orthogonal to t...

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Figure 7: A view of the alternated stacks along the b axis in (1c)₂(TCNQ).

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Figure 8: Detail of the overlap between donor and acceptor molecules in (1c)₂(TCNQ).

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Figure 9: Projection view along the a axis of the unit cell of (1c^+•)(FeCl₄⁻).

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Published 06 May 2015

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